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Browsing by Author "Bafaluy, Daniel"
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Copper-Catalyzed N-F Bond Activation for Uniform Intramolecular C-H Amination Yielding Pyrrolidines and Piperidines
Bafaluy, Daniel; Muñoz Molina, José María; Funes Ardoiz, Ignacio; Herold, Sebastian; Aguirre, Adiran J. de; Zhang, Hongwei; Maseras, Feliu; Rodríguez Belderraín, Tomás
; Pérez Romero, Pedro José
; Muñiz, Kilian (Wiley, 2019-06)
The dual function of the N-F bond as an effective oxidant and subsequent nitrogen source in intramolecular aliphatic C-H functionalization reactions is explored. Copper catalysis is demonstrated to exercise full regio- and ... -
Mechanistic Studies on the Synthesis of Pyrrolidines and Piperidines via Copper-Catalyzed Intramolecular C–H Amination
Muñoz Molina, José María; Bafaluy, Daniel; Funes Ardoiz, Ignacio; Aguirre, Adiran J. de; Maseras, Feliu; Rodríguez Belderraín, Tomás
; Pérez Romero, Pedro José
; Muñiz, Kilian (American Chemical Society, 2022)
We have recently developed a method for the synthesis of pyrrolidines and piperidines via intramolecular C–H amination of N-fluoride amides using [TpxCuL] complexes as precatalysts [Tpx = tris(pyrazolyl)borate ligand and ...